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Asymmetric organocatalysis: design of new organocatalysts and development of new methodologies

Grant number: 09/07281-0
Support type:Research Grants - Young Investigators Grants
Duration: November 01, 2009 - October 31, 2013
Field of knowledge:Physical Sciences and Mathematics - Chemistry
Principal Investigator:Márcio Weber Paixão
Grantee:Márcio Weber Paixão
Home Institution: Centro de Ciências Exatas e de Tecnologia (CCET). Universidade Federal de São Carlos (UFSCAR). São Carlos , SP, Brazil
Associated scholarship(s):12/04986-5 - Asymmetric organocatalysis: development of new methodologies and application in total synthesis, BP.PD
11/01055-8 - Organocatalysis: an excellent tool for the synthesis of bioactive molecules, BP.PD
10/10855-5 - Synthesis of triazole and structural analysis of Organochalcogen triazolics compounds, BP.DR
+ associated scholarships 11/01113-8 - Synthesis and biological evaluation of 1,4- and 1,5-disubstituted triazoles library, BP.IC
10/07664-3 - Synthesis and application of organocatalysts in asymmetric epoxidation reactions in order to synthesis of pheromones, BP.DR
09/14352-0 - Asymmetric organocatalysis: design of new organocatalysts and development of new methodologies, BP.JP - associated scholarships

Scientific publications (18)
(References retrieved automatically from Web of Science and SciELO through information on FAPESP grants and their corresponding numbers as mentioned in the publications by the authors)
LIMA, CAROLINA G. S.; SILVA, SANDRINA; GONCALVES, RICARDO H.; LEITE, EDSON R.; SCHWAB, RICARDO S.; CORREA, ARLENE G.; PAIXAO, MARCIO W. Highly Efficient and Magnetically Recoverable Niobium Nanocatalyst for the Multicomponent Biginelli Reaction. CHEMCATCHEM, v. 6, n. 12, p. 3455-3463, DEC 2014. Web of Science Citations: 21.
ECHEMENDIA, RADELL; CONCEPCION, ODETTE; MORALES, FIDEL E.; PAIXAO, MARCIO W.; RIVERA, DANIEL G. The Cu-I-catalyzed alkyne-azide cycloaddition as direct conjugation/cyclization method of peptides to steroids. Tetrahedron, v. 70, n. 20, p. 3297-3305, MAY 20 2014. Web of Science Citations: 13.
ALI, AKBAR; CORREA, ARLENE G.; ALVES, DIEGO; ZUKERMAN-SCHPECTOR, JULIO; WESTERMANN, BERNHARD; FERREIRA, MARCO A. B.; PAIXAO, MARCIO W. An efficient one-pot strategy for the highly regioselective metal-free synthesis of 1,4-disubstituted-1,2,3-triazoles. CHEMICAL COMMUNICATIONS, v. 50, n. 80, p. 11926-11929, 2014. Web of Science Citations: 44.
FEU, KARLA S.; DE LA TORRE, ALEXANDER F.; SILVA, SANDRINA; DE MORAES JUNIOR, MARCO A. F.; CORREA, ARLENE G.; PAIXAO, MARCIO W. Polyethylene glycol (PEG) as a reusable solvent medium for an asymmetric organocatalytic Michael addition. Application to the synthesis of bioactive compounds. GREEN CHEMISTRY, v. 16, n. 6, p. 3169-3174, 2014. Web of Science Citations: 30.
SANGI, DIEGO P.; MONTEIRO, JULIA L.; VANZOLINI, KENIA L.; CASS, QUEZIA B.; PAIXAO, MARCIO W.; CORREA, ARLENE G. Microwave-Assisted Synthesis of N-Heterocycles and Their Evaluation Using an Acetylcholinesterase Immobilized Capillary Reactor. Journal of the Brazilian Chemical Society, v. 25, n. 5, p. 887-889, Maio 2014. Web of Science Citations: 11.
DA SILVA, RODRIGO C.; DA SILVA, GUSTAVO P.; SANGI, DIEGO P.; PONTES, JOAO G. DE M.; FERREIRA, ANTONIO G.; CORREA, ARLENE G.; PAIXAO, MARCIO W. 1,1-Diamino-2-nitroethylenes as excellent hydrogen bond donor organocatalysts in the Michael addition of carbon-based nucleophiles to beta-nitrostyrenes. Tetrahedron, v. 69, n. 43, p. 9007-9012, OCT 28 2013. Web of Science Citations: 8.
DE LA TORRE, ALEXANDER F.; RIVERA, DANIEL G.; FERREIRA, MARCO A. B.; CORREA, ARLENE G.; PAIXAO, MARCIO W. Multicomponent Combinatorial Development and Conformational Analysis of Prolyl Peptide-Peptoid Hybrid Catalysts: Application in the Direct Asymmetric Michael Addition. Journal of Organic Chemistry, v. 78, n. 20, p. 10221-10232, OCT 18 2013. Web of Science Citations: 19.
NARAYANAPERUMAL, SENTHIL; RIVERA, DANIEL G.; SILVA, RODRIGO C.; PAIXAO, MARCIO W. Terpene-Derived Bifunctional Thioureas in Asymmetric Organocatalysis. CHEMCATCHEM, v. 5, n. 10, p. 2756-2773, OCT 2013. Web of Science Citations: 56.
FEU, KARLA SANTOS; DEOBALD, ANNA MARIA; NARAYANAPERUMAL, SENTHIL; CORREA, ARLENE G.; PAIXAO, MARCIO WEBER. An Eco-Friendly Asymmetric Organocatalytic Conjugate Addition of Malonates to ,-Unsaturated Aldehydes: Application on the Synthesis of Chiral Indoles. EUROPEAN JOURNAL OF ORGANIC CHEMISTRY, v. 2013, n. 26, p. 5917-5922, SEP 2013. Web of Science Citations: 12.
NARAYANAPERUMAL, SENTHIL; DA SILVA, RODRIGO CESAR; FEU, KARLA SANTOS; DE LA TORRE, ALEXANDER FERNANDEZ; CORREA, ARLENE G.; PAIXAO, MARCIO WEBER. Basic-functionalized recyclable ionic liquid catalyst: A solvent-free approach for Michael addition of 1,3-dicarbonyl compounds to nitroalkenes under ultrasound irradiation. ULTRASONICS SONOCHEMISTRY, v. 20, n. 3, p. 793-798, MAY 2013. Web of Science Citations: 24.
GODOI, MARCELO; RICARDO, EDUARDO W.; FRIZON, TIAGO E.; ROCHA, MANUELA S. T.; SINGH, DEVENDER; PAIXAO, MARCIO W.; BRAGA, ANTONIO LUIZ. An efficient synthesis of alkynyl selenides and tellurides from terminal acetylenes and diorganyl diselenides or ditellurides catalyzed by recyclable copper oxide nanopowder. Tetrahedron, v. 68, n. 51, p. 10426-10430, DEC 23 2012. Web of Science Citations: 19.
SEUS, NATALIA; GONCALVES, LOREN C.; DEOBALD, ANNA M.; SAVEGNAGO, LUCIELLI; ALVES, DIEGO; PAIXAO, MARCIO W. Synthesis of arylselanyl-1H-1,2,3-triazole-4-carboxylates by organocatalytic cycloaddition of azidophenyl arylselenides with beta-keto-esters. Tetrahedron, v. 68, n. 51, p. 10456-10463, DEC 23 2012. Web of Science Citations: 54.
NARAYANAPERUMAL, SENTHIL; DA SILVA, RODRIGO CESAR; MONTEIRO, JULIA L.; CORREA, ARLENE G.; PAIXAO, MARCIO W. Iron(III) Chloride Catalyzed Glycosylation of Peracylated Sugars with Allyl/Alkynyl Alcohols. Journal of the Brazilian Chemical Society, v. 23, n. 11, p. 1982-1988, NOV 2012. Web of Science Citations: 2.
SARAIVA, MAIARA T.; SEUS, NATALIA; DE SOUZA, DIEGO; RODRIGUES, OSCAR E. D.; PAIXAO, MARCIO W.; JACOB, RAQUEL G.; LENARDAO, EDER J.; PERIN, GELSON; ALVES, DIEGO. Synthesis of [(Arylselanyl)alkyl]-1,2,3-triazoles by Copper-Catalyzed 1,3-Dipolar Cycloaddition of (Arylselanyl)alkynes with Benzyl Azides. SYNTHESIS-STUTTGART, v. 44, n. 13, p. 1997-2004, JUL 2012. Web of Science Citations: 14.
DEOBALD, ANNA MARIA; CORREA, ARLENE G.; RIVERA, DANIEL G.; PAIXAO, MARCIO WEBER. Organocatalytic asymmetric epoxidation and tandem epoxidation/Passerini reaction under eco-friendly reaction conditions. ORGANIC & BIOMOLECULAR CHEMISTRY, v. 10, n. 38, p. 7681-7684, 2012. Web of Science Citations: 32.
DEOBALD, ANNA M.; CAMARGO, LEANDRO R. S.; ALVES, DIEGO; ZUKERMAN-SCHPECTOR, JULIO; CORREA, ARLENE G.; PAIXAO, MARCIO W. Click Chemistry: An Efficient Synthesis of Heterocycles Substituted with Steroids, Saponins, and Digitalis Analogues. SYNTHESIS-STUTTGART, n. 24, p. 4003-4010, DEC 2011. Web of Science Citations: 27.
GODOI, MARCELO; PAIXAO, MARCIO W.; BRAGA, ANTONIO L. Chiral organoselenium-transition-metal catalysts in asymmetric transformations. DALTON TRANSACTIONS, v. 40, n. 43, p. 11347-11355, 2011. Web of Science Citations: 71.
SCHWAB, RICARDO S.; SOARES, LETIERE C.; DORNELLES, LUCIANO; RODRIGUES, OSCAR E. D.; PAIXAO, MARCIO W.; GODOI, MARCELO; BRAGA, ANTONIO L. Chiral Chalcogen Peptides as Ligands for the Catalytic Enantioselective Aryl Transfer Reaction to Aldehydes. EUROPEAN JOURNAL OF ORGANIC CHEMISTRY, n. 19, p. 3574-3578, JUL 2010. Web of Science Citations: 31.

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