Advanced spectroscopy of novel nanomaterials

• Grant number: 13/16911-2
• Support type: Research Grants - Young Investigators Grants
• Duration: August 01, 2014 - July 31, 2019
• Field of knowledge: Physical Sciences and Mathematics - Physics - Condensed Matter Physics
• Principal Investigator: Lázaro Aurélio Padilha Junior
• Grantee: Lázaro Aurélio Padilha Junior
• Home Institution: Instituto de Física Gleb Wataghin (IFGW). Universidade Estadual de Campinas (UNICAMP). Campinas , SP, Brazil
• Assoc. researchers: Diogo Burigo Almeida
• Associated grant(s): 18/15574-6 - Advanced spectroscopy of nanomaterials: from ensemble to single-particle, AP.JP2; 17/21549-1 - Random lasers in semiconductor nanocrystals, AV.BR; 16/50011-7 - Two-dimensional spectroscopy of novel nanomaterials, AP.R SPRINT
• Associated scholarship(s): 15/06616-9 - Time-resolved spectroscopy in nanomaterials, BP.IC

Abstract

Recent advances on the development of new methods for synthesis of semiconductor nanostructures has allowed for better control of their optical and electronic properties. In those structures, quantum confinement changes the electronic structure changing existing and generating novel physical phenomena which are of interest not only for fundamental science but also for technological applications. This is the case of the enhanced multi-exciton generation rate in semiconductor quantum dots, which can be useful for application in generation-III solar panels. In this project, we propose to use ultrafast and nonlinear spectroscopy to study the dynamics of photoexcited carriers and the nonlinear optical response in nanostructured semiconductors. In particular, we will investigate multi-excitons interaction and multi-photon absorption in visible and near-infrared emitting nanoparticles which are candidates for applications on solar cells, 3D microscopy and telecommunications. Finally, this project will contribute to the expansion of ultrafast and nonlinear spectroscopy studies not only at UNICAMP but also, in the entire São Paulo State. (AU)

Scientific publications

(15)

(References retrieved automatically from Web of Science and SciELO through information on FAPESP grants and their corresponding numbers as mentioned in the publications by the authors)

ALO, ARTHUR; BARROS, LEONARDO W. T.; NAGAMINE, GABRIEL; VIEIRA, LUCAS B.; CHANG, JUN HYUK; JEONG, BYEONG GUK; BAE, WAN KI; PADILHA, LAZARO A. Simple Yet Effective Method to Determine Multiphoton Absorption Cross Section of Colloidal Semiconductor Nanocrystals. ACS PHOTONICS, v. 7, n. 7, p. 1806-1812, JUL 15 2020. Web of Science Citations: 0.

BONATO, LUIZ G.; MORAL, RAPHAEL F.; NAGAMINE, GABRIEL; ALO, ARTHUR; GERMINO, JOSE C.; DA SILVA, DOUGLAS S.; ALMEIDA, DIOGO B.; ZAGONEL, LUIZ F.; GALEMBECK, FERNANDO; PADILHA, LAZARO A.; NOGUEIRA, ANA FLAVIA. Revealing the Role of Tin(IV) Halides in the Anisotropic Growth of CsPbX3 Perovskite Nanoplates. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, MAY 2020. Web of Science Citations: 0.

LIU, ALBERT; BONATO, LUIZ G.; SESSA, FRANCESCO; ALMEIDA, DIOGO B.; ISELE, ERIK; NAGAMINE, GABRIEL; ZAGONEL, LUIZ F.; NOGUEIRA, ANA F.; PADILHA, LAZARO A.; CUNDIFF, STEVEN T. Effect of dimensionality on the optical absorption properties of CsPbI3 perovskite nanocrystals. Journal of Chemical Physics, v. 151, n. 19 NOV 21 2019. Web of Science Citations: 2.

LIU, ALBERT; ALMEIDA, DIOGO B.; BAE, WAN-KI; PADILHA, LAZARO A.; CUNDIFF, STEVEN T. Simultaneous Existence of Confined and Delocalized Vibrational Modes in Colloidal Quantum Dots. Journal of Physical Chemistry Letters, v. 10, n. 20, p. 6144-6150, OCT 17 2019. Web of Science Citations: 2.

LIU, A.; ALMEIDA, D. B.; BAE, W. K.; PADILHA, L. A.; CUNDIFF, S. T. Non-Markovian Exciton-Phonon Interactions in Core-Shell Colloidal Quantum Dots at Femtosecond Timescales. Physical Review Letters, v. 123, n. 5 AUG 2 2019. Web of Science Citations: 3.

TAZAWA, YUJIRO; HABISREUTINGER, SEVERIN N.; ZHANG, NANLIN; GREGORY, DANIEL A. F.; NAGAMINE, GABRIEL; KESAVA, SAMEER V.; MAZZOTTA, GIULIO; ASSENDER, HAZEL E.; RIEDE, MORITZ; PADILHA, LAZARO A.; NICHOLAS, ROBIN J.; WATT, ANDREW A. R. Carbon Nanotubes for Quantum Dot Photovoltaics with Enhanced Light Management and Charge Transport. ACS PHOTONICS, v. 5, n. 12, p. 4854-4863, DEC 2018. Web of Science Citations: 1.

CHANG, JUN HYUK; PARK, PHILIP; JUNG, HEEYOUNG; JEONG, BYEONG GUK; HAHM, DONGHYO; NAGAMINE, GABRIEL; KO, JONGKUK; CHO, JINHAN; PADILHA, LAZARO A.; LEE, DOH C.; LEE, CHANGHEE; CHAR, KOOKHEON; BAE, WAN KI. Unraveling the Origin of Operational Instability of Quantum Dot Based Light-Emitting Diodes. ACS NANO, v. 12, n. 10, p. 10231-10239, OCT 2018. Web of Science Citations: 11.

NAGAMINE, GABRIEL; NUNCIARONI, HENRIQUE B.; MCDANIEL, HUNTER; EFROS, ALEXANDER L.; DE BRITO CRUZ, CARLOS H.; PADILHA, LAZARO A. Evidence of Band-Edge Hole Levels Inversion in Spherical CuInS2 Quantum Dots. Nano Letters, v. 18, n. 10, p. 6353-6359, OCT 2018. Web of Science Citations: 10.

NAGAMINE, GABRIEL; ROCHA, JAQUELINE O.; BONATO, LUIZ G.; NOGUEIRA, ANA F.; ZAHARIEVA, ZHANET; WATT, ANDREW A. R.; DE BRITO CRUZ, CARLOS H.; PADILHA, LAZARO A. Two-Photon Absorption and Two-Photon-Induced Gain in Perovskite Quantum Dots. Journal of Physical Chemistry Letters, v. 9, n. 12, p. 3478-3484, JUN 21 2018. Web of Science Citations: 18.

PELEGATI, VITOR B.; KYOTOKU, BERNARDO B. C.; PADILHA, LAZARO A.; CESAR, CARLOS L. Six-wave mixing coherent anti-Stokes Raman scattering microscopy. BIOMEDICAL OPTICS EXPRESS, v. 9, n. 5, p. 2407-2417, MAY 1 2018. Web of Science Citations: 1.

BARROS, LEONARDO W. T.; CARDOSO, THIAGO A. S.; BIHLMEIER, ANGELA; WAGNER, DANNY; KOELMEL, DOMINIK K.; HOERNER, ANNA; BRAESE, STEFAN; CRUZ, CARLOS H. BRITO; PADILHA, LAZARO A. Two-photon absorption in a series of 2,6-disubstituted BODIPY dyes. Physical Chemistry Chemical Physics, v. 19, n. 32, p. 21683-21690, AUG 28 2017. Web of Science Citations: 7.

ROSA, HENRIQUE G.; CASTANEDA, JUAN A.; BRITO CRUZ, CARLOS H.; PADILHA, LAZARO A.; GOMES, JOSE C. V.; THOROH DE SOUZA, EUNEZIO A.; FRAGNITO, HUGO L. Controlled stacking of graphene monolayer saturable absorbers for ultrashort pulse generation in erbium-doped fiber lasers. OPTICAL MATERIALS EXPRESS, v. 7, n. 7, p. 2528-2537, JUL 1 2017. Web of Science Citations: 4.

YASSITEPE, EMRE; YANG, ZHENYU; VOZNYY, OLEKSANDR; KIM, YOUNGHOON; WALTERS, GRANT; CASTANEDA, JUAN ANDRES; KANJANABOOS, PONGSAKORN; YUAN, MINGJIAN; GONG, XIWEN; FAN, FENGJIA; PAN, JUN; HOOGLAND, SJOERD; COMIN, RICCARDO; BAKR, OSMAN M.; PADILHA, LAZARO A.; NOGUEIRA, ANA F.; SARGENT, EDWARD H. Amine-Free Synthesis of Cesium Lead Halide Perovskite Quantum Dots for Efficient Light-Emitting Diodes. ADVANCED FUNCTIONAL MATERIALS, v. 26, n. 47, p. 8757-8763, DEC 20 2016. Web of Science Citations: 94.

CASTANEDA, JUAN A.; NAGAMINE, GABRIEL; YASSITEPE, EMRE; BONATO, LUIZ G.; VOZNYY, OLEKSANDR; HOOGLAND, SJOERD; NOGUEIRA, ANA F.; SARGENT, EDWARD H.; BRITO CRUZ, CARLOS H.; PADILHA, LAZARO A. Efficient Biexciton Interaction in Perovskite Quantum Dots Under Weak and Strong Confinement. ACS NANO, v. 10, n. 9, p. 8603-8609, SEP 2016. Web of Science Citations: 45.

KOELMEL, DOMINIK K.; HOERNER, ANNA; CASTANEDA, JUAN A.; FERENCZ, JULIO A. P.; BIHLMEIER, ANGELA; NIEGER, MARTIN; BRAESE, STEFAN; PADILHA, LAZARO A. Linear and Nonlinear Optical Spectroscopy of Fluoroalkylated BODIPY Dyes. Journal of Physical Chemistry C, v. 120, n. 8, p. 4538-4545, MAR 3 2016. Web of Science Citations: 15.

Academic Publications

(References retrieved automatically from State of São Paulo Research Institutions)

JUNIOR, Lázaro Aurélio Padilha. Revealing the electronic structure of nanomaterials using advanced optical spectroscopy. 2017. Master's Dissertation.