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Innovative proposal for N2 2 capturing in Liquid Argon using the Li-FAU molecular Sieve

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Cardoso, Dilson ; Segreto, Ettore ; Cruz, Ivana ; da Silva, Edilene Deise ; Zapelini, Iago William ; Goncalves, Rosembergue G. ; Freitas, G. S. ; Caffer, Ana Maria ; Souza, J. C. ; Christovam, D. S. ; Mazali, Italo O. ; Reis, Cristhiane ; Assaf, Elisabete ; Assaf, Jose Mansur ; Soccol, Renato ; Bianchi, Pedro ; Wiederhecker, Gustavo ; Noriler, Dirceu ; dos Santos, Cezar Rodrigo Aguiar ; Brant, Krystal ; Fontes, Magda ; Oliveira Jr, N. F. ; Correia, Daniel ; Frandini, Heriques ; Demolin, Frederico ; Augusto, Andre ; Doubnik, Roza ; Adamowski, Mark ; Montanari, David ; Alegre, Thiago P. M. ; Adriano, Cris ; Machado, Ana Amelia ; Pagliuso, P. G.
Número total de Autores: 33
Tipo de documento: Artigo Científico
Fonte: Journal of Instrumentation; v. 19, n. 8, p. 9-pg., 2024-08-01.
Resumo

In this work, we unveil the potential of nitrogen (N-2) adsorption from Liquid Argon (LAr) through the molecular sieves (zeolites) Li-FAU Adsorbents. We report detailed studies about N-2 gas adsorption at T = 89 K using a commercial Micromeritics ASAP-2420 equipment and N-2 purification from LAr using the Purification Cryostat (PuLArC) at IFGW/Unicamp. We argue that the N-2 adsorption by the Li-FAU is possible thanks to the stronger interaction of N-2 with the lithium cations present in zeolite Li-FAU. In fact, the experiments performed in PuLArC have unequivocally shown that the Li-FAU adsorbent was capable of capturing N-2, reducing a N-2 contamination of 20-50 ppm to 0.1-1.0 ppm in 1-2 hours of circulation time in LAr for several runs. This result demonstrated the great potential of the Li-FAU adsorbent for N-2 capturing in LAr and invoke further tests of this material in larger scale LAr cryostats in order to confirm the innovative proposal of using the Li-FAU molecular sieve in replacement of Molecular Sieve 4A, currently used in LAr cryostats for neutrino experiments. (AU)

Processo FAPESP: 20/01609-2 - Otimização dos procedimentos de purificação, regeneração e condensação de argônio para instalações de grande escala
Beneficiário:Pascoal Jose Giglio Pagliuso
Modalidade de apoio: Auxílio à Pesquisa - Regular