Physical and chemical characteristics of plasma-activated water generated by hybrid dielectric barrier discharge and gliding arc discharge

Autor(es)

Neto, Nilton F. Azevedo ; Miranda, Felipe S. ; Moreira Jr, Pedro W. P. ; Gomes, Marcelo P. ; Alves Jr, Clodomiro ; Koga-Ito, Cristiane Y. ; Pessoa, Rodrigo S.

• Tipo de documento: Artigo Científico
• Fonte: JOURNAL OF PHYSICS D-APPLIED PHYSICS; v. 57, n. 41, p. 15-pg., 2024-10-18.

Resumo

This research explores the synergistic application of Dielectric Barrier Discharge (DBD) and Gliding Arc Plasma Jet (GAPJ) in a Hybrid Plasma Discharge (HPD) setup for enhanced water activation. The HPD system demonstrated balanced and sustained generation of reactive oxygen and nitrogen species (RONS), maintaining efficiency at higher specific input energy (SIE) values. Comparative analyses with DBD and GAPJ systems highlighted the superior performance of the HPD system in generating RONS and modifying water's molecular structure. Key observations included a decrease in water's pH and an increase in oxidation-reduction potential, total dissolved solids, and conductivity, stabilizing beyond 5 l min-1 airflow and 10 min of treatment. UV-Vis spectroscopy identified nitrites, nitrates, hydrogen peroxide, and nitrous acid, while Raman spectroscopy captured shifts in vibrational modes, particularly in librational and O-H stretching bands. These changes correlated with alterations in reactive species concentrations and pH levels. Overall, the HPD system emerged as a versatile and efficient approach for generating plasma-activated water, suitable for applications in microbial deactivation, surface sterilization, and electrocatalytic process optimization, offering stable and continuous production of reactive species across a range of SIE values. (AU)

• Processo FAPESP: 19/05856-7 - Aplicações de plasmas atmosféricos não-térmicos na odontologia: da bancada para a clínica
• Beneficiário: Cristiane Yumi Koga Ito
• Modalidade de apoio: Auxílio à Pesquisa - Temático
• Processo FAPESP: 21/14181-3 - Desenvolvimento e estudo de um sistema de plasma gerado por descarga de barreira dielétrica (DBD) para ativação contínua de líquidos aplicados em tratamentos odontológicos.
• Beneficiário: Felipe de Souza Miranda
• Modalidade de apoio: Bolsas no Brasil - Pós-Doutorado
• Processo FAPESP: 23/02268-2 - Geração e caracterização de diferentes líquidos ativados com plasma para aplicação no tratamento endodôntico
• Beneficiário: Nilton Francelosi Azevedo Neto
• Modalidade de apoio: Bolsas no Brasil - Pós-Doutorado