Purification and preparation of TlBr crystals for room temperature radiation detector applications

Autor(es)

Oliveira, I. B. ; Costa, F. E. ; Chubaci, J. F. D. ; Hamada, M. M. ^[4]

• Tipo de documento: Artigo Científico
• Fonte: IEEE Transactions on Nuclear Science; v. 51, n. 3, p. 1224-1228, 2004.
• Área do conhecimento: Engenharias - Engenharia Nuclear
• Assunto(s): Radiação (energia radiante) Semicondutores (físico-química)

Resumo

Thallium bromide (TlBr) is a semiconductor compound with a high atomic number and a wide bandgap, being a very promising material to be used as room temperature radiation detectors. In this work, commercial TlBr powder was used for growing crystals for detector applications. To reduce impurities, this material was purified by the zone refining technique. Trace impurities at ppb/ppm level were analyzed using inductively coupled plasma mass spectroscopy (ICP-MS). The efficiency of the purification was evaluated through studies of the decrease impurities concentrations in the TlBr powder and in the purified materials. The crystal quality was verified by X-ray diffraction (XRD). To evaluate the crystal as a semiconductor detector, systematic measurements of the transmittance, resistivity, and the radiation response (/sup 241/Am, /sup 57/Co, /sup 125/I, and /sup 133/Ba) gamma rays were carried out. (AU)

• Processo FAPESP: 01/09049-5 - Desenvolvimento do cristal semicondutor de brometo de tálio para aplicações como detector de radiação fotodetector
• Beneficiário: Icimone Braga de Oliveira
• Modalidade de apoio: Bolsas no Brasil - Doutorado