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Theoretical study of molecules in astrophysical environments

Grant number:19/07671-4
Support Opportunities:Regular Research Grants
Start date: September 01, 2019
End date: August 31, 2021
Field of knowledge:Physical Sciences and Mathematics - Physics - Atomic and Molecular Physics
Principal Investigator:Rene Felipe Keidel Spada
Grantee:Rene Felipe Keidel Spada
Host Institution: Divisão de Ciências Fundamentais (IEF). Instituto Tecnológico de Aeronáutica (ITA). São José dos Campos , SP, Brazil
City of the host institution:São José dos Campos

Abstract

During this proposal period, properties of diatomic and polyatomic molecules of astrophysical interest will be calculated. For diatomic molecules spectroscopic properties will be obtained, first using multireferential electronic structure methods for the calculation of electronic potential surfaces, and then the nuclear equation will be solved numerically. These results will be used to obtain the rovibrational energy levels of these molecules, Franck-Condon factors (related to the transition probabilities) and the Einstein coefficients (related to the decay time of each transition). The formation of polyatomic molecules in interstellar environments will be studied also. For such a study, highly correlated ab initio methodologies and approximations for density functional theory will be used to describe the thermochemical properties of elementary reactions present in the mechanism of formation of such molecules. The rate constants of such reactions will be obtained by variation of transition state theory with approximations for tunneling effects. (AU)

Articles published in Agência FAPESP Newsletter about the research grant:
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VEICULO: TITULO (DATA)
VEICULO: TITULO (DATA)

Scientific publications (15)
(The scientific publications listed on this page originate from the Web of Science or SciELO databases. Their authors have cited FAPESP grant or fellowship project numbers awarded to Principal Investigators or Fellowship Recipients, whether or not they are among the authors. This information is collected automatically and retrieved directly from those bibliometric databases.)
ALVES, ESDRAS; FRANCO, MAURICIO P.; PILLING, SERGIO; MACHADO, FRANCISCO B. C.; SPADA, RENE F. K.. The influence of the environment in chemical reactivity: the HCOOH formation from the H2O + CO reaction. Journal of Molecular Modeling, v. 27, n. 9, . (19/25105-6, 19/07671-4)
SILVA, SILVIA G. S.; VICHIETTI, RAFAEL M.; HAIDUKE, ROBERTO L. A.; MACHADO, FRANCISCO B. C.; SPADA, RENE F. K.. Methanol and glycolaldehyde production from formaldehyde in massive star-forming regions. Monthly Notices of the Royal Astronomical Society, v. 497, n. 4, p. 4486-4494, . (19/07671-4, 18/05691-5, 14/23714-1)
VICHIETTI, RAFAEL M.; SPADA, RENE F. K.; MACHADO, FRANCISCO B. C.; HAIDUKE, ROBERTO L. A.. Accurate rate constants for elementary reactions of molecular hydrogen and carbon monoxide mixtures and the role of the H-2 rich environment. Journal of Molecular Modeling, v. 28, n. 8, p. 9-pg., . (18/05691-5, 14/23714-1, 19/25105-6, 10/18743-1, 19/07671-4)
FRANCO, MAURICIO P.; CARVALHO, BEATRIZ B.; RIBEIRO, MARCOS A.; SPADA, RENE F. K.. Evaluation of N-binding through N1, N2 or N3 of 4-R-1,2,3-Triazolate to [CuCO](+) Complexes. CHEMISTRYSELECT, v. 7, n. 10, p. 5-pg., . (19/07671-4)
SPADA, RENE F. K.; FRANCO, MAURICIO P.; NIEMAN, REED; AQUINO, ADELIA J. A.; SHEPARD, RON; PLASSER, FELIX; LISCHKA, HANS. Spin-density calculation via the graphical unitary group approach. Molecular Physics, v. N/A, p. 17-pg., . (19/07671-4)
VICHIETTI, RAFAEL; SPADA, RENE F. K.; DA SILVA, ALBERICO B. F.; MACHADO, FRANCISCO B. C.; HAIDUKE, ROBERTO L. A.. A Proposal for the Mechanism of the CH + CO2 Reaction. ACS OMEGA, v. 4, n. 18, p. 17843-17849, . (19/07671-4, 17/07707-3, 10/18743-1, 18/05691-5, 14/23714-1)
NUNEZ-REYES, DIANAILYS; HICKSON, KEVIN M.; LOISON, JEAN-CHRISTOPHE; SPADA, RENE F. K.; VICHIETTI, RAFAEL M.; MACHADO, FRANCISCO B. C.; HAIDUKE, ROBERTO L. A.. Tunneling Enhancement of the Gas-Phase CH + CO2 Reaction at Low Temperature. Journal of Physical Chemistry A, v. 124, n. 51, p. 10717-10725, . (19/25105-6, 19/07671-4, 14/23714-1, 18/05691-5)
LISCHKA, HANS; SHEPARD, RON; MUELLER, THOMAS; SZALAY, PETER G.; PITZER, RUSSELL M.; AQUINO, ADELIA J. A.; ARAUJO DO NASCIMENTO, MAYZZA M.; BARBATTI, MARIO; BELCHER, LACHLAN T.; BLAUDEAU, JEAN-PHILIPPE; et al. The generality of the GUGA MRCI approach in COLUMBUS for treating complex quantum chemistry. Journal of Chemical Physics, v. 152, n. 13, . (19/07671-4, 17/50157-4)
RODRIGUES, AUGUSTO R.; BELCHER, LACHLAN T.; SPADA, RENE F. K.. Thermochemical and kinetic investigation of the hydrazine borane as an alternative to hydrazine: The N2H4BH3+H reactional system. Chemical Physics Letters, v. 828, p. 8-pg., . (19/07671-4)
VIEIRA, ISABELA S.; FREIRE, PAULO T. C.; SPADA, RENE F. K.. Thermochemical and kinetics investigation of the CH2CN + CN system leading to NCCH2CN. Chemical Physics Letters, v. 815, p. 7-pg., . (19/07671-4)
LAKSHMANAN, SANDHIYA; SPADA, RENE F. K.; MACHADO, FRANCISCO B. C.; HASE, WILLIAM L.. Potential Energy Curves for Formation of the CH2O2 Criegee Intermediate on the (CH2)-C-3 + O-3(2) Singlet and Triplet Potential Energy Surfaces. Journal of Physical Chemistry A, v. 123, n. 41, p. 8968-8975, . (19/07671-4, 17/07707-3)
VICHIETTI, R. M.; SPADA, R. F. K.; DA SILVA, A. B. F.; MACHADO, F. B. C.; HAIDUKE, R. L. A.. Could HCN Be Responsible for the Formamide Synthesis in Earth?s Primitive Atmosphere?. ASTROPHYSICAL JOURNAL SUPPLEMENT SERIES, v. 245, n. 1, . (19/07671-4, 17/07707-3, 14/23714-1, 18/05691-5, 10/18743-1)
VIEIRA, ISABELA S.; LIMA, LINEIDE A.; FREIRE, PAULO T. C.; SPADA, RENE F. K.. Thermochemical and kinetics investigation of elementary reactions to produce acetonitrile in Titan's atmosphere. Chemical Physics Letters, v. 871, p. 7-pg., . (19/07671-4)
NUNEZ-REYES, DIANAILYS; HICKSON, KEVIN M.; LOISON, JEAN-CHRISTOPHE; SPADA, RENE F. K.; VICHIETTI, RAFAEL M.; MACHADO, FRANCISCO B. C.; HAIDUKE, ROBERTO L. A.. Tunneling Enhancement of the Gas-Phase CH + CO2 Reaction at Low Temperature. Journal of Physical Chemistry A, v. 124, n. 51, p. 9-pg., . (19/25105-6, 14/23714-1, 18/05691-5, 19/07671-4)
PINTO, CESAR H.; VIEIRA, ISABELA S.; SPADA, RENE F. K.. Elementary reactions for glycine production in hot and dense interstellarmedia from CH3COOH, HCOOH, and NH2CH. Journal of Molecular Modeling, v. 31, n. 1, p. 13-pg., . (19/07671-4)