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Proposal for Zeeman slowing of Rb-2 molecules in a supersonic beam, inducing internal cooling

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Author(s):
Torres, Manuel Alejandro Lefran ; Passagem, Henry Fernandes ; Fernandez, David Rodriguez ; da Costa Paul, Eduardo ; Casique, Cristian Adan Mojica ; Dulieu, Olivier ; Bouloufa-Maafa, Nadia ; Marcassa, Luis Gustavo
Total Authors: 8
Document type: Journal article
Source: JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS; v. 56, n. 6, p. 10-pg., 2023-03-28.
Abstract

We present a theoretical proposal on Zeeman slowing of a Rb-2 supersonic beam, relying on transitions between rovibrational levels of the X-1 sigma(+)(g) electronic ground-state and the B-1 Pi(u) electronic excited state. Translational cooling is induced by optical transitions from v(X) (SIC) 13, J(X )(SIC) 13 to v(B) = 0 involving P (J(B) = J(X) - 1) and Q (J(B) = J(X)) branches. This is achieved by shaping the spectrum of broadband laser sources, in addition to two single-frequency laser sources addressing the X-1 sigma(+)(g) (v(X) = 2, 3, J(X) = 1) -> B-1 Pi(u)(v(B) = 0, J(B) = 1) transitions. Our Monte-Carlo simulations indicate that the velocity of the molecules can be slowed from 500 m s(-1) down to a few m s(-1 )by a Zeeman slower with a 1.2 m length, after scattering about 150 000 photons. At the end of the slowing process, half of the molecules are internally cooled, predicted to be in the v(X) = 2, 3, J(X) = 1 ground-state levels. A final optical pumping step transferring the population to the v(X) = 0, J(X )= 1 ground-state level could produce a molecular beam exiting the Zeeman slower which is cold in all the translational, vibrational, and rotational degrees of freedom. Such an approach could potentially be a great interest for cooling down a large class of molecular species. (AU)

FAPESP's process: 19/23510-0 - Optical cavity for Rydberg atom experiments
Grantee:David Rodríguez Fernández
Support Opportunities: Scholarships in Brazil - Master
FAPESP's process: 19/10971-0 - Optical cavities for trapping of atoms and molecules
Grantee:Luis Gustavo Marcassa
Support Opportunities: Regular Research Grants
FAPESP's process: 21/04107-0 - Collisions in a Cold Trapped Molecular Sample in a well-defined quantum state: COCOTRAMOS
Grantee:Luis Gustavo Marcassa
Support Opportunities: Research Projects - Thematic Grants
FAPESP's process: 18/06835-0 - Magneto optical trap of Rb2 molecules and colissional studies
Grantee:Manuel Alejandro Lefrán Torres
Support Opportunities: Scholarships in Brazil - Doctorate