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Orbitally defined field-induced electronic state in a Kondo lattice

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Author(s):
Lesseux, G. G. ; Sakai, H. ; Hattori, T. ; Tokunaga, Y. ; Kambe, S. ; Kuhns, P. L. ; Reyes, A. P. ; Thompson, J. D. ; Pagliuso, P. G. ; Urbano, R. R.
Total Authors: 10
Document type: Journal article
Source: PHYSICAL REVIEW B; v. 101, n. 16, p. 6-pg., 2020-04-10.
Abstract

CeRhIn5 is a Kondo-lattice prototype in which a magnetic field B* similar or equal to 31 T induces an abrupt Fermi-surface (FS) reconstruction and pronounced in-plane electrical transport anisotropy all within its antiferromagnetic state. Though the antiferromagnetic order at zero field is well understood, the origin of an emergent state at B* remains unknown due to challenges inherent to probing states microscopically at high fields. Here we report low-temperature nuclear magnetic resonance (NMR) measurements revealing a pronounced decrease in the In-115 formal Knight shift, without changes in crystal or magnetic structures, of CeRhIn5 at fields (parallel to c) spanning B*. We discuss the emergent state above B* in terms of a change in Ce's 4f orbitals that arises from field-induced evolution of crystal-electric field (CEF) energy levels. This change in orbital character enhances hybridization between the 4f and the conduction electrons that leads ultimately to an itinerant quantum-critical point at B-c0 similar or equal to 50 T. (AU)

FAPESP's process: 12/05903-6 - Nuclear magnetic resonance of novel complex and advanced materials in condensed matter physics
Grantee:Ricardo Rodrigues Urbano
Support Opportunities: Research Grants - Young Investigators Grants
FAPESP's process: 17/10581-1 - Emergent phenomena in reduced dimension systems
Grantee:Pascoal Jose Giglio Pagliuso
Support Opportunities: Special Projects
FAPESP's process: 12/04870-7 - Studies of novel complex and advanced materials
Grantee:Pascoal Jose Giglio Pagliuso
Support Opportunities: Research Projects - Thematic Grants