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(Reference retrieved automatically from Web of Science through information on FAPESP grant and its corresponding number as mentioned in the publication by the authors.)

Combined external pressure and Cu-substitution studies on BaFe2As2 single crystals

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Author(s):
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Piva, M. M. [1, 2] ; Besser, M. [2] ; Mydeen, K. [2] ; Garitezi, T. M. [1] ; Rosa, P. F. S. [1, 3] ; Adriano, C. [1] ; Grant, T. [3] ; Fisk, Z. [3] ; Urbano, R. R. [1] ; Nicklas, M. [2] ; Pagliuso, P. G. [1]
Total Authors: 11
Affiliation:
[1] Univ Estadual Campinas, Inst Fis Gleb Wataghin, BR-13083859 Campinas, SP - Brazil
[2] Max Planck Inst Chem Phys Solids, D-01187 Dresden - Germany
[3] Univ Calif Irvine, Irvine, CA 92697 - USA
Total Affiliations: 3
Document type: Journal article
Source: JOURNAL OF PHYSICS-CONDENSED MATTER; v. 27, n. 14 APR 15 2015.
Web of Science Citations: 1
Abstract

We report a combined study of external pressure and Cu-substitution on BaFe2As2 single crystals grown by the in-flux technique. At ambient pressure, the Cu-substitution is known to suppress the spin density wave (SDW) phase in pure BaFe2As2 (T-SDW approximate to 140 K) and to induce a superconducting (SC) dome with a maximum transition temperature T-c(max) similar or equal to 4.2 K. This T-c(max) is much lower than the T-c similar to 15-28 K achieved in the case of Ru, Ni and Co substitutions. Such a lower T-c is attributed to a Cu2+ magnetic pair-breaking effect. The latter is strongly suppressed by applied pressure, as shown herein, T-c can be significantly enhanced by applying high pressures. In this work, we investigated the pressure effects on Cu2+ magnetic pair-breaking in the BaFe2-xCuxAs2 series. Around the optimal concentration (x(opd) = 0.11), all samples showed a substantial increase of T-c as a function of pressure. Yet for those samples with a slightly higher doping level (over-doped regime), T-c presented a dome-like shape with maximum T-c similar or equal to 8K. Remarkably interesting, the under-doped samples, e.g. x = 0.02 display a maximum pressure induced T-c similar or equal to 30 K which is comparable to the maximum T-c's found for the pure compound under external pressures. Furthermore, the magnetoresistance effect as a function of pressure in the normal state of the x = 0.02 sample also presented an evolution consistent with the screening of the Cu2+ local moments. These findings demonstrate that the Cu2+ magnetic pair-breaking effect is completely suppressed by applying pressure in the low concentration regime of Cu2+ substituted BaFe2As2. (AU)

FAPESP's process: 09/09247-3 - Investigation of pressure induced ordered states in novel complex materials.
Grantee:Cris Adriano
Support Opportunities: Scholarships in Brazil - Post-Doctoral
FAPESP's process: 13/20181-0 - Evolution of topological Kondo insulating behavior in Sm1xRxB6 (r = Sr, Yb)
Grantee:Priscila Ferrari Silveira Rosa
Support Opportunities: Scholarships abroad - Research Internship - Post-doctor
FAPESP's process: 12/04870-7 - Studies of novel complex and advanced materials
Grantee:Pascoal Jose Giglio Pagliuso
Support Opportunities: Research Projects - Thematic Grants
FAPESP's process: 13/10833-0 - Synthesis and caracterization of single crystaline PrCuBi2 intermetallic compound
Grantee:Mário Moda Piva
Support Opportunities: Scholarships in Brazil - Scientific Initiation
FAPESP's process: 12/05903-6 - Nuclear magnetic resonance of novel complex and advanced materials in condensed matter physics
Grantee:Ricardo Rodrigues Urbano
Support Opportunities: Research Grants - Young Investigators Grants
FAPESP's process: 09/10264-0 - Study of intermetalic compounds for thermoelectrical applications by x-ray diffraction
Grantee:José Renato Linares Mardegan
Support Opportunities: Scholarships in Brazil - Doctorate
FAPESP's process: 11/19924-2 - Study and development of advanced novel materials: electronic, magnetic and nanostructured: an interdisciplinary approach
Grantee:Carlos Rettori
Support Opportunities: Research Projects - Thematic Grants
FAPESP's process: 11/01564-0 - Materials sciences on complex and advanced systems
Grantee:Pascoal Jose Giglio Pagliuso
Support Opportunities: Scholarships abroad - Research
FAPESP's process: 11/23650-5 - Investigation of band structure and Fermi surface in advanced complex materials studied by angle-resolved photoemission spectroscopy
Grantee:Cris Adriano
Support Opportunities: Scholarships abroad - Research Internship - Post-doctor