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Nodeless time-reversal symmetry breaking in the centrosymmetric superconductor Sc(5)Co(4)Si(10 )probed by muon-spin spectroscopy

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Bhattacharyya, A. ; Lees, M. R. ; Panda, K. ; Ferreira, P. P. ; Dorini, T. T. ; Gaudry, Emilie ; Eleno, L. T. F. ; Anand, V. K. ; Sannigrahi, J. ; Biswas, P. K. ; Tripathi, R. ; Adroja, D. T.
Total Authors: 12
Document type: Journal article
Source: PHYSICAL REVIEW MATERIALS; v. 6, n. 6, p. 10-pg., 2022-06-15.
Abstract

We investigate the superconducting properties of Sc5Co4Si10 using low-temperature resistivity, magnetization, heat capacity, and muon-spin rotation and relaxation (mu SR) measurements. We find that Sc5Co4Si10 exhibits type-II superconductivity with a superconducting transition temperature T-C = 3.5(1)K. The temperature dependence of the superfluid density obtained from transverse-field mu SR spectra is best modeled using an isotropic Bardeen-Cooper-Schrieffer type s-wave gap symmetry with 2 Delta/k(B)T(C) = 2.84(2). However, the zero-field muon-spin relaxation rate reveals the appearance of a spontaneous magnetic field below T-C, indicating that time-reversal symmetry (TRS) is broken in the superconducting state. Although this behavior is commonly associated with nonunitary or mixed singlet-triplet pairing, our group-theoretical analysis of the Ginzburg-Landau free energy alongside density functional theory calculations indicates that unconventional mechanisms are pretty unlikely. Therefore, we have hypothesized that TRS breaking may occur via a conventional electron-phonon process. (AU)

FAPESP's process: 20/08258-0 - Ab initio study of superconducting and topological systems
Grantee:Pedro Nunes Ferreira
Support Opportunities: Scholarships in Brazil - Doctorate
FAPESP's process: 19/05005-7 - Computational Materials Laboratory for the ab initio study of the stability of intermetallic compounds
Grantee:Luiz Tadeu Fernandes Eleno
Support Opportunities: Regular Research Grants