Evolution of the Fe-Co magnetism and magnetic proximity effects in alternate Fe/Co monolayers on nonmagnetic Cu3Au(001)

Author(s)

Cabral, L. ; Macedo, W. A. A. ; da Silva, E. Z.

• Document type: Journal article
• Source: PHYSICAL REVIEW B; v. 106, n. 21, p. 12-pg., 2022-12-23.

Abstract

Magnetic heterostructures with ferromagnetic/nonmagmetic interfaces are very interesting materials due to the possibility to switch the magnetization, to control the induced magnetic moment, and also due to interfacial effects. The tuning of the spin-orbit coupling in magnetic materials allows engineering new spintronic devices. Using density functional theory, the induced local magnetic moments in copper and gold surface atoms of Cu3Au(001) due to the deposited alternate magnetic Fe and Co monolayers were studied. To observe the tuning mechanism, the spin density of the FeCo/Cu3Au(001) as a function of the number of deposited magnetic monolayers was extensively investigated. The Fe/Co deposition induces a hybridization between electronic states of the magnetic and nonmagnetic interface atoms, generating a broadening in d bands of the deposited material, engineering the magnetic moments of the interface atoms. This observed hybridization elucidates the charge variation in the interface atoms for stacking sequences starting with Fe or with Co as the first magnetic layer in direct contact with the Cu3Au(001) substrate. By performing the spin-charge density calculations, we demonstrated that this magnetic induction occurs only for the nonmagnetic Cu-Au atoms at the Cu3Au(001) surface. (AU)

• FAPESP's process: 17/26105-4 - Multi-user equipment approved in grant 2016/23891-6 high performace computational cluster
• Grantee: Alex Antonelli
• Support Opportunities: Multi-user Equipment Program
• FAPESP's process: 16/23891-6 - Computer modeling of condensed matter
• Grantee: Alex Antonelli
• Support Opportunities: Research Projects - Thematic Grants
• FAPESP's process: 13/07296-2 - CDMF - Center for the Development of Functional Materials
• Grantee: Elson Longo da Silva
• Support Opportunities: Research Grants - Research, Innovation and Dissemination Centers - RIDC
• FAPESP's process: 18/20729-9 - Formation of Ag Nanoparticles by Laser Irradiation: An ab inicio Investigation
• Grantee: Luis Antônio Cabral
• Support Opportunities: Scholarships in Brazil - Post-Doctoral