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The impact of different flexible substrates on the photothermal reduction quality of graphene oxide

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Author(s):
Bonando, Matheus Guitti ; Moreira, Gabriel Monte Mor ; Fernandes, Nathalia Maria Moraes ; Steinberg, David ; Cadore, Alisson Ronieri ; Silva, Cecilia de Carvalho Castro ; Saito, Lucia Akemi Miyazato
Total Authors: 7
Document type: Journal article
Source: NANOSCALE ADVANCES; v. 6, n. 18, p. 7-pg., 2024-07-17.
Abstract

In this work, we demonstrate the impact of the photothermal reduction quality of graphene oxide (GO), which is affected by the material composition, roughness, and thermal properties of the membrane substrates. We show high efficiency reduced graphene oxide (rGO) conversion by applying a 405 nm pulsed laser in ambient conditions onto different flexible substrates. Three filter membranes, such as nylon, cellulose acetate, and nitrocellulose, are used as rGO thin film substrates, achieving sheet resistance of 51 +/- 2, 58 +/- 3, and 620 +/- 40 Omega sq-1, respectively, which has been the lowest resistance reported in ambient conditions. Finally, we demonstrate that such flexible materials can be applied as temperature sensors ranging from 35 degrees C to 100 degrees C. The best sensitivity is achieved using nylon membranes, showing a smoother rGO surface and lower defect density. This work shows the lowest reported sheet resistances obtained by laser-reduced graphene oxide in ambient conditions for nylon and cellulose acetate substrates (51 +/- 2 and 58 +/- 3 Omega sq-1) by optimizing the photothermal reduction of graphene oxide. (AU)

FAPESP's process: 22/08932-9 - Light-emitting diodes (LEDs) based on two-dimensional Van der Waals heterostructures for visible telecom and sensing applications
Grantee:Eunezio Antonio de Souza
Support Opportunities: Regular Research Grants