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Ultra-confined plasmons reveal moiré patterns in a twisted bilayer graphene-talc heterostructure

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Author(s):
Barbosa, Tiago C. ; Chaves, Andre J. ; Freitas, Raul O. ; Campos, Leonardo C. ; Barcelos, Ingrid D.
Total Authors: 5
Document type: Journal article
Source: NANOSCALE; v. 17, n. 15, p. 8-pg., 2025-02-12.
Abstract

This work investigates the plasmonic properties of a twisted bilayer graphene (TBG) and talc heterostructure. Talc, a naturally occurring phyllosilicate, promotes p-type charging of graphene, supporting high charge mobility and strong interaction between graphene plasmons and talc's phonon polaritons. This interaction results in the formation of surface plasmon-phonon polariton (SP3) modes, which are detected using infrared scattering-type scanning near-field optical microscopy (IR s-SNOM) at room temperature. Notably, without the need for electrostatic gating, our study reveals confinement of SP3 modes in a TBG-talc heterostructure and a transition from surface plasmonic waves to the emergence of moir & eacute; superlattices, characterized by reflections at domain walls. These findings provide fresh insights into the coupling mechanisms in hybrid materials and suggest promising applications in nanoscale optoelectronics. (AU)

FAPESP's process: 22/02901-4 - Nano-optics of polaritons in two-dimensional crystals and at the metal/dielectric interface in the mid-to-far infrared
Grantee:Francisco Carlos Barbosa Maia
Support Opportunities: Research Grants - Initial Project
FAPESP's process: 19/14017-9 - From excitons waves to THz-phonons: 2Ds materials nano-optics via synchrotron infrared nanospectroscopy
Grantee:Raul de Oliveira Freitas
Support Opportunities: Research Grants - Young Investigators Grants