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Separation of critical metals through supported liquid membrane: evaluation of synergistic interaction between organophosphorus and membranes

Grant number: 23/01032-5
Support Opportunities:Scholarships abroad - Research Internship - Post-doctor
Start date: June 01, 2023
End date: May 31, 2024
Field of knowledge:Engineering - Chemical Engineering
Principal Investigator:Denise Crocce Romano Espinosa
Grantee:Amilton Barbosa Botelho Junior
Supervisor: William Abraham Tarpeh
Host Institution: Escola Politécnica (EP). Universidade de São Paulo (USP). São Paulo , SP, Brazil
Institution abroad: Stanford University, United States  
Associated to the scholarship:21/14842-0 - Elucidation of the organometallic complexation mechanism between organic extractants and rare earth elements, BP.PD

Abstract

Critical metals have a severe risk of interruption in the supply chain in the short and medium term. The leading economies worldwide have rare earth elements, Li and Co, in their list of critical metals. These elements are critical to producing technologies in strategic sectors, as in the case of renewable energy, e-mobility, defense, and aerospace, and they are essential to achieving a net zero society. The processes to obtain these metals may be designed and carried out considering the aspects of sustainable development, which includes low energy consumption and fewer CO2 emissions. The hydrometallurgical process (aqueous route) includes leaching and separation/purification steps and represents great sustainable advances, including producing high-pure products. The critical step of the process is separation/purification, in which the presence of contaminants negatively impacts the production of high-pure products. Moreover, the rare earth elements are chemically similar and represent a challenge to overcome. Membrane technology for the separation of metals represents the next generation of separation/purification techniques, which represents the knowledge beyond the state-of-art. The current project aimed the study membrane separation of rare earth elements, Li and Co, using supported liquid membrane separation. Different phosphinic organic extractants, such as Cyanex 272, Cyanex 923, and D2EHPA, will be explored. The organic extractants will be placed in contact with a membrane before experiments. The effect of the concentration of organic extractant, stripping solution, and metallic ions will be evaluated. The synthetic solutions to be treated will simulate the real solutions from the extraction of critical metals from primary and secondary sources. This project will be focused on the separation mechanism through the membrane supported with different phosphinic acids as organic extractants. (AU)

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Scientific publications (18)
(References retrieved automatically from Web of Science and SciELO through information on FAPESP grants and their corresponding numbers as mentioned in the publications by the authors)
DIAS, MARIA EDUARDA DE MELO GOLCALVES; TENORIO, JORGE ALBERTO SOARES; ESPINOSA, DENISE CROCCE ROMANO; BOTELHO JUNIOR, AMILTON BARBOSA. Recycling of Li-Ion Batteries: Recovery of Critical Metals by Hydrometallurgy. JOM, v. N/A, p. 12-pg., . (20/00493-0, 23/01032-5, 21/14842-0, 19/11866-5)
BOTELHO JUNIOR, AMILTON BARBOSA; ABELS, KRISTEN; ESPINOSA, DENISE CROCCE ROMANO; TARPEH, WILLIAM A.. Lithium Extraction by Electrodialysis: Effect of Co-Occurring Ions for Application in Brine Processing. Journal of the Electrochemical Society, v. 172, n. 2, p. 10-pg., . (23/01032-5, 19/11866-5, 21/14842-0)
LIMA, ANASTASSIA MARIAH NUNES DE OLIVEIRA; ESPINOSA, DENISE CROCCE ROMANO; GOBO, LUCIANA ASSIS; KUMOTO, ELIO AUGUSTO; BOTELHO JUNIOR, AMILTON BARBOSA; TENORIO, JORGE ALBERTO SOARES. Study of the behaviour of cations in leaching of NCA lithium-ion batteries by electrodialysis. ENVIRONMENTAL TECHNOLOGY, v. N/A, p. 12-pg., . (19/11866-5, 23/01032-5, 20/00493-0, 21/14842-0)
CHEJE MACHACA, DARWIN MICHELL; BOTELHO JR, AMILTON BARBOSA; DE CARVALHO, THAMYRES CARDOSO; TENORIO, JORGE ALBERTO SOARES; ESPINOSA, DENISE CROCCE ROMANO. Hydrometallurgical processing of chalcopyrite: A review of leaching techniques. INTERNATIONAL JOURNAL OF MINERALS METALLURGY AND MATERIALS, v. 31, n. 12, p. 19-pg., . (21/14842-0, 20/00493-0, 19/11866-5, 23/01032-5)
ABELS, KRISTEN; JUNIOR, AMILTON BARBOSA BOTELHO; CHEN, XI; TARPEH, WILLIAM A.. Ligand content and driving force effects on ion-ion permselectivity in ligand-functionalized membranes. JOURNAL OF MEMBRANE SCIENCE, v. 714, p. 11-pg., . (19/11866-5, 23/01032-5)
BOTELHO, AMILTON BARBOSA, JR.; DA SILVA, DAVID VASCONCELOS; NUNES DE OLIVEIRA LIMA, ANASTASSIA MARIAH; DE OLIVEIRA, RAFAEL PIUMATTI; GOBO, LUCIANA ASSIS; KUMOTO, ELIO AUGUSTO; FERRARESE, ANDRE; SOARES TENORIO, JORGE ALBERTO; ROMANO ESPINOSA, DENISE CROCCE. LAREX-Tupy Process: Recycling of Li-Ion Batteries from Electric Vehicles by Hydrometallurgical Route Towards Circular Economy. TMS 2024 153RD ANNUAL MEETING & EXHIBITION: SUPPLEMENTAL PROCEEDINGS, v. N/A, p. 8-pg., . (19/11866-5, 23/01032-5, 20/00493-0, 21/14842-0)
PREMATHILAKE, DILSHAN SANDARUWAN; AMBAYE, TEKLIT GEBREGIORGIS; BOTELHO JR, AMILTON BARBOSA; LIMA, ANA TERESA MACAS; ESPINOSA, DENISE CROCCE ROMANO; VACCARI, MENTORE. Comparative environmental and economic assessment of emerging hydrometallurgical recycling technologies for Li-ion battery cathodes. SUSTAINABLE PRODUCTION AND CONSUMPTION, v. 51, p. 18-pg., . (21/14842-0, 20/00493-0, 19/11866-5, 23/01032-5)
BOTELHO JUNIOR, AMILTON BARBOSA; MIYASHITA, ANA CAROLINA; SOARES TENORIO, JORGE ALBERTO; ROMANO ESPINOSA, DENISE CROCCE. Separation of Critical Metals Using Supported Liquid Membranes PTFE-Cyanex 272. RARE METAL TECHNOLOGY 2024, v. N/A, p. 8-pg., . (21/14842-0, 20/00493-0, 19/11866-5, 23/01032-5)
MARTINS, FLAVIO PINHEIRO; ALMARAZ, SOFIA DE-LEON; BOTELHO JUNIOR, AMILTON BARBOSA; AZZARO-PANTEL, CATHERINE; PARIKH, PRITI. Hydrogen and the sustainable development goals: Synergies and trade-offs. RENEWABLE & SUSTAINABLE ENERGY REVIEWS, v. 204, p. 11-pg., . (21/14842-0, 20/00493-0, 19/11866-5, 23/01032-5)
DOS SANTOS, LUIS HENRIQUE DO NASCIMENTO; PEREIRA, BARBARA DA ROCHA; ROSSET, MORGANA; ESPINOSA, DENISE CROCCE ROMANO; BOTELHO JUNIOR, AMILTON BARBOSA. High purity alumina production by leaching-ion exchange process: Design and flowchart proposal. MINERALS ENGINEERING, v. 217, p. 11-pg., . (21/14842-0, 19/11866-5, 23/01032-5)
BOTELHO, AMILTON BARBOSA; DA SILVA, NATALIA OLIM MARTINS; TENORIO, JORGE ALBERTO SOARES; ESPINOSA, DENISE CROCCE ROMANO. Structure Investigation of La, Y, and Nd Complexes in Solvent Extraction Process with Liquid Phosphine Oxide, Phosphinic Acid, and Amine Extractants. METALS, v. 13, n. 8, p. 16-pg., . (19/11866-5, 21/14842-0, 23/01032-5)
LIMA, ANASTASSIA MARIAH NUNES DE OLIVEIRA; DA LUZ, VILSON CONRADO; ESPINOSA, DENISE CROCCE ROMANO; GOBO, LUCIANA ASSIS; KUMOTO, ELIO AUGUSTO; BOTELHO JUNIOR, AMILTON BARBOSA; TENORIO, JORGE ALBERTO SOARES. Electrodialysis as a route for separating metals from NCA-type automotive lithium-ion batteries. JOURNAL OF CLEANER PRODUCTION, v. 527, p. 12-pg., . (23/01032-5, 20/00493-0, 21/14842-0, 19/11866-5)
BRAZ, VITOR MOOR PINHEIRO; VACCARI, MENTORE; ESPINOSA, DENISE CROCCE ROMANO; TENORIO, JORGE ALBERTO SOARES; BOTELHO JUNIOR, AMILTON BARBOSA. Effect of Iron Oxidation State on Solvent Extraction Scandium Extraction Process from Bauxite Residue and Life Cycle Assessment. JOM, v. 77, n. 11, p. 13-pg., . (23/01032-5, 21/14842-0, 22/16507-6, 19/11866-5, 23/15491-1)
BOTELHO JUNIOR, AMILTON BARBOSA; LIMA DALVI, GUILHERME DE FREITAS; CAVALCANTE, VINICIUS SMITH; MIYASHITA, ANA CAROLINA; SOARES TENORIO, JORGE ALBERTO; ROMANO ESPINOSA, DENISE CROCCE. Supported Liquid Membranes for Separation of Critical Raw Metals. TMS 2025 154TH ANNUAL MEETING & EXHIBITION SUPPLEMENTAL PROCEEDINGS, v. N/A, p. 9-pg., . (23/01032-5, 20/00493-0, 21/14842-0, 19/11866-5)
GUIMARAES, LUCAS FONSECA; TENORIO, JORGE ALBERTO SOARES; VACCARI, MENTORE; ESPINOSA, DENISE CROCCE ROMANO; BOTELHO JUNIOR, AMILTON BARBOSA. Characterization of Lithium-Ion Batteries from Recycling Perspective towards Circular Economy. MINERALS, v. 14, n. 9, p. 21-pg., . (21/14842-0, 20/00493-0, 19/11866-5, 23/01032-5)
COOMBS, ORISA Z.; JOO, TAIGYU; BOTELHO JUNIOR, AMILTON BARBOSA; CHALISE, DIVYA; TARPEH, WILLIAM A.. Prototyping and modelling a photovoltaic-thermal electrochemical stripping system for distributed urine nitrogen recovery. NATURE WATER, v. 3, n. 8, p. 22-pg., . (23/01032-5, 19/11866-5)
PETRAGLIA, FERNANDA FAJARDO NACIF; VINHAL, JONATHAN TENORIO; BOTELHO JUNIOR, AMILTON BARBOSA; ESPINOSA, DENISE CROCCE ROMANO. Recycling of permanent magnets: A perspective for application of organic acids and ionic liquids towards eco-friendly process. JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, v. 12, n. 6, p. 10-pg., . (21/14842-0, 19/11866-5, 23/01032-5, 22/01159-2)
BOTELHO JUNIOR, AMILTON BARBOSA; MARTINS, FLAVIO PINHEIRO; CEZARINO, LUCIANA ORANGES; LIBONI, LARA BARTOCCI; SOARES TENORIO, JORGE ALBERTO; ROMANO ESPINOSA, DENISE CROCCE. The sustainable development goals, urban mining, and the circular economy. EXTRACTIVE INDUSTRIES AND SOCIETY-AN INTERNATIONAL JOURNAL, v. 16, p. 14-pg., . (21/14842-0, 19/11866-5, 23/01032-5)