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(Reference retrieved automatically from Web of Science through information on FAPESP grant and its corresponding number as mentioned in the publication by the authors.)

Complex magnetic behavior along the Gdln (NixCu1-x)(4) (0.00 <= x <= 1.00) series of compounds

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Author(s):
Mercena, S. G. [1] ; Mendonca, E. C. [1] ; Meneses, C. T. [1] ; Silva, L. S. [1, 2] ; Duque, J. G. S. [3, 1] ; Jesus, C. B. R. [3, 1] ; Souza, J. C. [3] ; Pagliuso, P. G. [3]
Total Authors: 8
Affiliation:
[1] Univ Fed Sergipe, Programa Posgrad Fis, Campus Prof Jose Aluisio de Campos, BR-49100000 Sao Cristovao, SE - Brazil
[2] IFTO, Inst Fed Tocantins, Campus Colinas Do Tocantins, BR-77760000 Colinas Do Tocantins, TO - Brazil
[3] Univ Estadual Campinas, Inst Fis Gleb Wataghin, BR-13083970 Campinas, SP - Brazil
Total Affiliations: 3
Document type: Journal article
Source: Journal of Applied Physics; v. 125, n. 6 FEB 14 2019.
Web of Science Citations: 1
Abstract

In this work, structural, magnetic, and local properties of GdIn(NixCu1-x)(4) (0.00 <= x <= 1.00) samples synthesized via the flux method are investigated by means of X-ray, magnetization, specific heat, and electron spin resonance measurements. The analysis of X-ray powder diffraction data taken at room temperature reveals that all samples belong to the cubic space group (Cl5b-type structure) with lattice parameters, a, ranging from 7.08 < a < 7.23 angstrom. Interestingly, the analysis of both T-dependence magnetic susceptibility and MvsH loops indicates a gradual transition from antiferromagnetic to ferromagnetic ground states as a function of the Ni-doping. The transition temperatures are confirmed via specific heat measurements. Finally, electron spin resonance data taken in the temperature range of 100 <= T <= 300 K show a single Dysonian line shape, which is characteristic of a metallic environment. A nearly T-independent g-value was observed and the value was concentration independent. Besides, the doped samples show an increase of the residual linewidth, which can be linked with the chemical disorder introduced by the Ni-doping. Our results are discussed considering the bottleneck and multiple band effects on the Gd3+ spin dynamics in this series and their implication in the magnetic frustration observed in these materials. Published under license by AIP Publishing. (AU)

FAPESP's process: 18/11364-7 - Magnetic properties of complex systems with non-trivial topology
Grantee:Jean Carlo Souza
Support type: Scholarships in Brazil - Doctorate
FAPESP's process: 12/04870-7 - Studies of novel complex and advanced materials
Grantee:Pascoal Jose Giglio Pagliuso
Support type: Research Projects - Thematic Grants
FAPESP's process: 17/10581-1 - Emergent phenomena in reduced dimension systems
Grantee:Pascoal Jose Giglio Pagliuso
Support type: Research Projects - Thematic Grants