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(Reference retrieved automatically from Web of Science through information on FAPESP grant and its corresponding number as mentioned in the publication by the authors.)

Enhanced optical cross-section of radiation induced defect centers under plasmon resonance conditions: Shifting stimulation wavelength of optically stimulated luminescence dosimeters

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Author(s):
Isikawa, M. M. [1] ; Assuncao, A. C. A. [1] ; Guidelli, O. Baffa E. J. [1]
Total Authors: 3
Affiliation:
[1] Univ Sao Paulo, Dept Fis, FFCLRP, BR-14040901 Ribeirao Preto, SP - Brazil
Total Affiliations: 1
Document type: Journal article
Source: Journal of Luminescence; v. 231, MAR 2021.
Web of Science Citations: 1
Abstract

Plasmon-enhanced luminescence is an important tool for development of advanced sensing technologies but the mechanisms originating these enhancements are still in debate. In this work, we investigate plasmon-enhanced luminescence mechanisms using the Optically Stimulated Luminescence (OSL) from defect centers in X-ray irradiated sodium chloride nanocrystals deposited on silver nanoparticle (AgNP) films with varying plasmon properties upon blue, green, and red OSL stimulation. Although the absolute OSL intensity for NaCl crystals is higher upon blue stimulation, under plasmon resonance conditions, higher absolute OSL intensity occurs upon green stimulation and the largest OSL enhancements are observed by employing red stimulation. These results suggest that, as long as the OSL stimulation wavelength is well tuned with the film plasmon band, plasmonic coupling does not depend on the trap depth and that the largest luminescence enhancements are achieved in spectral regions where the optical cross-sections of the defect centers are smaller. In terms of radiation dosimetry applications, this result allows to shift the stimulation wavelength farther from the OSL emission window, improving the signal to noise ratio and the dose assessment sensitivity and accuracy. (AU)

FAPESP's process: 13/07699-0 - Research, Innovation and Dissemination Center for Neuromathematics - NeuroMat
Grantee:Oswaldo Baffa Filho
Support Opportunities: Research Grants - Research, Innovation and Dissemination Centers - RIDC