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Fabrication and characterization of devices and systems based on hybrid nanomembranes

Abstract

Nanomembranes are freestanding nanostructures with mescopic thicknesses and with lateral dimensions in the macroscopic range. By strain and stress engineering inside the nanomembranes, self-assembled three-dimensional (3D) structures, such as microtubes and micro-ribbons, can be formed. Since the patterning methods used for manufacturing the nanomembranes are the same ones employed in standard microfabrication processes, the creation of 3D devices based on microtubes and micro-ribbons is a typical case where bottom-up and top-down methods are combined to give rise to novel technologies. In this proposal, we intend to implement and consolidate the processes of synthesis, patterning and characterization of hybrid organic/inorganic nanomembranes, as well as their application in electronic, electrochemical and microfluidic devices at LNNano/CNPEM. Three categories of demonstrators are proposed in order to solidify the fabrication processes: a) Ultra-compact elements, such as supercapacitors and organic transistors, which use the mechanical flexibility of the nanomembranes to reduce the devices footprint. b) Sensors that exploit the quasi-bidimensional nature of the nanomembranes to improve their performance and to incorporate different functionalities. c) Hybrid organic/inorganic heterojunctions, that uses the mechanical flexibility of the nanomembrane, associated with their patterning and integration capabilities, to generate robust devices on-a-chip exhibiting novel physical and chemical properties. (AU)

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Scientific publications (39)
(References retrieved automatically from Web of Science and SciELO through information on FAPESP grants and their corresponding numbers as mentioned in the publications by the authors)
SILVA, RICARDO M. L.; MERCES, LEANDRO; BOF BUFON, CARLOS C.. Temperature-Independent Polarization of Ultrathin Phthalocyanine-Based Hybrid Organic/Inorganic Heterojunctions. ACS APPLIED MATERIALS & INTERFACES, v. 12, n. 26, p. 29556-29565, . (18/18136-0, 14/25979-2, 14/50906-9)
VELLO, TATIANA PARRA; ALBANO, LUIZ GUSTAVO SIMAO; DOS SANTOS, THAMIRIS CESCON; COLLETTI, JULIA CANTOVITZ; SANTOS BATISTA, CARLOS VINICIUS; LEME, VITORIA FERNANDES CINTRA; DOS SANTOS, THAMIRIS COSTA; MIGUEL, MARIA PAULA DIAS CARNEIRO; DE CAMARGO, DAVI HENRIQUE STARNINI; BOF BUFON, CARLOS CESAR. Electrical Conductivity Boost: In Situ Polypyrrole Polymerization in Monolithically Integrated Surface-Supported Metal-Organic Framework Templates. SMALL, v. N/A, p. 14-pg., . (17/02317-2, 14/50906-9, 16/25346-5, 19/01561-2, 14/25979-2, 17/25553-3)
PAULIN, JOAO V.; BAYRAM, SINAN; GRAEFF, CARLOS F. O.; BUFON, CARLOS C. B.. Exploring the Charge Transport of a Natural Eumelanin for Sustainable Technologies. ACS APPLIED BIO MATERIALS, v. 6, n. 9, p. 5-pg., . (17/02317-2, 20/15869-6, 14/50906-9, 14/25979-2)
MINATOGAU FERRO, LETICIA MARIE; DE BARROS, ANERISE; ZAPAROLI FALSETTI, LUIS OTAVIO; CORREA, CATIA CRISPILHO; MERCES, LEANDRO; BOF BUFON, CARLOS CESAR. Highly efficient electrochemical energy conversion in a 3D hollow microenvironment: towards on-a-chip sensor applications. JOURNAL OF MATERIALS CHEMISTRY A, v. 8, n. 38, p. 11-pg., . (18/18136-0, 14/50906-9, 17/21117-4, 14/25979-2)
SANTOS BATISTA, CARLOS VINICIUS; MERCES, LEANDRO; RODRIGUES COSTA, CARLOS ALBERTO; STARNINI DE CAMARGO, DAVI HENRIQUE; BOF BUFON, CARLOS CESAR. High-Performance Ultrathin Molecular Rectifying Diodes Based on Organic/Inorganic Interface Engineering. ADVANCED FUNCTIONAL MATERIALS, v. 32, n. 6, . (14/50906-9, 14/25979-2, 19/10188-3, 18/18136-0)
DE ANDRADE, DENISE MARIA; MERCES, LEANDRO; NAWAZ, ALI; BUFON, CARLOS CESAR BOF. Pushing On-Chip Photosensitivity Forward Using Edge-Driven Vertical Organic Phototransistors. ACS APPLIED ELECTRONIC MATERIALS, v. 5, n. 6, p. 10-pg., . (19/14949-9, 17/02317-2, 14/50906-9, 18/18136-0, 14/25979-2)
VELLO, TATIANA P.; DA SILVA, LARISSA M. B.; SILVA, GUSTAVO O.; DE CAMARGO, DAVI H. S.; CORREA, CATIA C.; BOF BUFON, CARLOS C.. Hybrid organic/inorganic interfaces as reversible label-free platform for direct monitoring of biochemical interactions. BIOSENSORS & BIOELECTRONICS, v. 87, p. 209-215, . (14/25979-2, 13/22127-2)
MERCES, LEANDRO; DE OLIVEIRA, RAFAEL FURLAN; STARNINI DE CAMARGO, DAVI HENRIQUE; BOF BUFON, CARLOS CESAR. Long-Range Coherent Tunneling in Physisorbed Molecular Ensembles. Journal of Physical Chemistry C, v. 121, n. 31, p. 16673-16681, . (14/25979-2)
PETRINI, PAULA A.; SILVA, RICARDO M. L.; DE OLIVEIRA, RAFAEL F.; MERCES, LEANDRO; BOF BUFON, CARLOS C.. Hybrid nanomembrane-based capacitors for the determination of the dielectric constant of semiconducting molecular ensembles. Nanotechnology, v. 29, n. 26, . (14/25979-2)
DE OLIVEIRA, RAFAEL FURLAN; MERCES, LEANDRO; MARQUES, FELIPE; TEIXEIRA-NETO, ERICO; STARNINI DE CAMARGO, DAVI HENRIQUE; BOF BUFON, CARLOS CESAR. Single-Electron Charging Effects in Hybrid Organic/Inorganic Nanomembrane-Based Junctions. Journal of Physical Chemistry C, v. 122, n. 23, p. 12131-12139, . (14/25979-2)
TORIKAI, KLEYTON; DE OLIVEIRA, RAFAEL FURLAN; STARNINI DE CAMARGO, DAVI H.; BOF BUFON, CARLOS C.. Low-Voltage, Flexible, and Self-Encapsulated Ultracompact Organic Thin-Film Transistors Based on Nanomembranes. Nano Letters, v. 18, n. 9, p. 5552-5561, . (14/25979-2)
DAMASCENO, SERGIO; CORREA, CATIA CRISPILHO; GOUVEIA, RUBIA FIGUEREDO; STRAUSS, MATHIAS; BOF BUFON, CARLOS CESAR; SANTHIAGO, MURILO. Delayed Capillary Flow of Elastomers: An Efficient Method for Fabrication and Nanofunctionalization of Flexible, Foldable, Twistable, and Stretchable Electrodes from Pyrolyzed Paper. ADVANCED ELECTRONIC MATERIALS, v. 6, n. 1, . (14/25979-2, 13/22127-2)
SANTHIAGO, MURILO; STRAUSS, MATHIAS; PEREIRA, MARIANE P.; CHAGAS, ANDREIA S.; BUFON, CARLOS C. B.. Direct Drawing Method of Graphite onto Paper for High-Performance Flexible Electrochemical Sensors. ACS APPLIED MATERIALS & INTERFACES, v. 9, n. 13, p. 11959-11966, . (14/25979-2, 09/54066-7, 13/22127-2)
LOPES, CAROLINA SERGI; MERCES, LEANDRO; DE OLIVEIRA, RAFAEL FURLAN; STARNINI DE CAMARGO, DAVI HENRIQUE; BOF BUFON, CARLOS CESAR. Rectification ratio and direction controlled by temperature in copper phthalocyanine ensemble molecular diodes. NANOSCALE, v. 12, n. 18, p. 10001-10009, . (16/25346-5, 14/25979-2, 14/50906-9, 18/18136-0)
VELLO, TATIANA PARRA; STRAUSS, MATHIAS; RODRIGUES COSTA, CARLOS ALBERTO; CORREA, CATIA CRISPILHO; BOF BUFON, CARLOS CESAR. Deterministic control of surface mounted metal-organic framework growth orientation on metallic and insulating surfaces. Physical Chemistry Chemical Physics, v. 22, n. 10, p. 5839-5846, . (14/25979-2, 16/25346-5, 14/50906-9)
NAWAZ, ALI; MERCES, LEANDRO; DE ANDRADE, DENISE M.; DE CAMARGO, DAVI H. S.; BOF BUFON, CARLOS C.. Edge-driven nanomembrane-based vertical organic transistors showing a multi-sensing capability. NATURE COMMUNICATIONS, v. 11, n. 1, . (14/25979-2, 16/25346-5, 14/50906-9, 18/18136-0)
JIMENEZ, MAWIN J. M.; DE OLIVEIRA, RAFAEL F.; BUFON, CARLOS CESAR B.; PEREIRA-DA-SILVA, MARCELO A.; RODRIGUES, VARLEI; GOBBI, ANGELO L.; PIAZZETTA, MARIA H. O.; ALVAREZ, FERNANDO; CESAR, CARLOS LENZ; RIUL JR, ANTONIO. Enhanced mobility and controlled transparency in multilayered reduced graphene oxide quantum dots: a charge transport study. Nanotechnology, v. 30, n. 27, . (14/25979-2, 14/03691-7)
SANTHIAGO, MURILO; DA COSTA, PRISCILA G.; PEREIRA, MARIANE P.; CORREA, CATIA C.; DE MORAIS, VITCORIA B.; BUFON, CARLOS C. B.. Versatile and Robust Integrated Sensors To Locally Assess Humidity Changes in Fully Enclosed Paper-Based Devices. ACS APPLIED MATERIALS & INTERFACES, v. 10, n. 41, p. 35631-35638, . (14/25979-2, 13/22127-2)
ALBANO, LUIZ G. S.; DE CAMARGO, DAVI H. S.; SCHLEDER, GABRIEL R.; DEEKE, SAMANTHA G.; VELLO, TATIANA P.; PALERMO, LEIRSON D.; CORREA, CATIA C.; FAZZIO, ADALBERTO; WOELL, CHRISTOF; BUFON, CARLOS C. B.. Room-Temperature Negative Differential Resistance in Surface-Supported Metal-Organic Framework Vertical Heterojunctions. SMALL, v. 17, n. 35, . (17/18139-6, 14/25979-2, 16/25346-5, 14/50906-9, 19/01561-2, 17/02317-2, 17/25553-3)
FERRO, LETICIA M. M.; MERCES, LEANDRO; DE CAMARGO, DAVI H. S.; BUFON, CARLOS C. B.. Ultrahigh-Gain Organic Electrochemical Transistor Chemosensors Based on Self-Curled Nanomembranes. Advanced Materials, v. 33, n. 29, . (14/25979-2, 13/22127-2, 14/50906-9, 18/18136-0, 17/21117-4)
PAULIN, JOAO V.; PEREIRA, MARIANE P.; BREGADIOLLI, BRUNA A.; CACHANESKI-LOPES, JOAO P.; GRAEFF, CARLOS F. O.; BATAGIN-NETO, AUGUSTO; BUFON, CARLOS C. B.. Controlling ions and electrons in aqueous solution: an alternative point of view of the charge-transport behavior of eumelanin-inspired material. JOURNAL OF MATERIALS CHEMISTRY C, v. 11, n. 18, p. 12-pg., . (17/02317-2, 17/07627-0, 14/50906-9, 20/15869-6, 14/25979-2)
BARCELOS, INGRID D.; CADORE, ALISSON R.; ALENCAR, ANANIAS B.; MAIA, FRANCISCO C. B.; MANIA, EDRIAN; OLIVEIRA, RAFAEL F.; BUFON, CARLOS C. B.; MALACHIAS, ANGELO; FREITAS, RAUL O.; MOREIRA, ROBERTO L.; et al. Infrared Fingerprints of Natural 2D Talc and Plasmon-Phonon Coupling in Graphene-Talc Heterostructures. ACS PHOTONICS, v. 5, n. 5, SI, p. 1912-1918, . (14/25979-2)
FERRO, LETICIA M. M.; MERCES, LEANDRO; DE CAMARGO, DAVI H. S.; BUFON, CARLOS C. B.. Ultrahigh-Gain Organic Electrochemical Transistor Chemosensors Based on Self-Curled Nanomembranes. Advanced Materials, . (17/21117-4, 13/22127-2, 14/25979-2, 14/50906-9, 18/18136-0)
SANTHIAGO, MURILO; CORREA, CATIA C.; BERNARDES, JULIANA S.; PEREIRA, MARIANE P.; OLIVEIRA, LETICIA J. M.; STRAUSS, MATHIAS; BUFON, CARLOS C. B.. Flexible and Foldable Fully-Printed Carbon Black Conductive Nanostructures on Paper for High-Performance Electronic, Electrochemical, and Wearable Devices. ACS APPLIED MATERIALS & INTERFACES, v. 9, n. 28, p. 24365-24372, . (14/25979-2, 09/54066-7, 13/22127-2)
MERCES, LEANDRO; DE OLIVEIRA, RAFAEL FURLAN; GOMES, HENRIQUE LEONEL; BOF BUFON, CARLOS CESAR. The role of the electrode configuration on the electrical properties of small-molecule semiconductor thin-films. ORGANIC ELECTRONICS, v. 49, p. 107-113, . (14/25979-2)
VELLO, TATIANA P.; DE OLIVEIRA, RAFAEL F.; SILVA, GUSTAVO O.; DE CAMARGO, DAVI H. S.; BUFON, CARLOS C. B.. A simple capacitive method to evaluate ethanol fuel samples. SCIENTIFIC REPORTS, v. 7, . (14/25979-2, 13/22127-2)
JIMENEZ, MAWIN J. M.; OLIVEIRA, RAFAEL F.; ALMEIDA, TIAGO P.; HENSEL FERREIRA, RAFAEL C.; BUFON, CARLOS CESAR B.; RODRIGUES, VARLEI; PEREIRA-DA-SILVA, MARCELO A.; GOBBI, ANGELO L.; PIAZZETTA, MARIA H. O.; RIUL, JR., ANTONIO. Charge carrier transport in defective reduced graphene oxide as quantum dots and nanoplatelets in multilayer films. Nanotechnology, v. 28, n. 49, . (14/25979-2, 14/03691-7)
POZZOLI, GUILHERME L.; MERCES, LEANDRO; YASSITEPE, EMRE; DE MORAIS, VITORIA B.; DE CAMARGO, DAVI H. S.; BUFON, CARLOS C. BOF. Charge Transport and Gradient Doping in Nanostructured Polypyrrole Films for Applications in Photocurrent Generation. ACS APPLIED NANO MATERIALS, v. 3, n. 3, p. 3060-3070, . (18/18136-0, 14/25979-2, 14/50906-9)
ALBANO, LUIZ G. S.; VELLO, TATIANA P.; DE CAMARGO, DAVI H. S.; DA SILVA, RICARDO M. L.; PADILHA, ANTONIO C. M.; FAZZIO, ADALBERTO; BUFON, CARLOS C. B.. Ambipolar Resistive Switching in an Ultrathin Surface-Supported Metal-Organic Framework Vertical Heterojunction. Nano Letters, v. 20, n. 2, p. 1080-1088, . (17/25553-3, 14/50906-9, 17/02317-2, 16/25346-5, 14/25979-2, 18/05565-0)
JIMENEZ, MAWIN J. M.; DE OLIVEIRA, RAFAEL F.; SHIMIZU, FLAVIO M.; BUFON, CARLOS CESAR B.; RODRIGUES, VARLEI; GOBBI, ANGELO L.; PIAZZETTA, MARIA H. O.; RIUL JR, ANTONIO. Poole-Frenkel emission on functionalized, multilayered-packed reduced graphene oxide nanoplatelets. Nanotechnology, v. 29, n. 50, . (14/25979-2, 14/03691-7)
DE MORAIS, VITORIA BRITO; CORREA, CATIA CRISPILHO; LANZONI, EVANDRO MARTIN; RODRIGUES COSTA, CARLOS ALBERTO; BOF BUFON, CARLOS CESAR; SANTHIAGO, MURILO. Wearable binary cooperative polypyrrole nanofilms for chemical mapping on skin. JOURNAL OF MATERIALS CHEMISTRY A, v. 7, n. 10, p. 5227-5233, . (14/25979-2, 13/22127-2)
PAULIN, JOAO V.; ALBANO, LUIZ G. S.; CAMARGO, DAVI H. S.; PEREIRA, MARIANE P.; BREGADIOLLI, BRUNA A.; GRAEFF, CARLOS F. O.; BUFON, CARLOS C. B.. Eumelanin-based multisensory platform: A case of study for photolithographic patterning. APPLIED MATERIALS TODAY, v. 28, p. 9-pg., . (20/15869-6, 17/07627-0, 14/25979-2, 17/02317-2, 17/25553-3)
BAR, JACIARA; DE BARROS, ANERISE; DE CAMARGO, DAVI H. S.; PEREIRA, MARIANE P.; MERCES, LEANDRO; SHIMIZU, FLAVIO MAKOTO; SIGOLI, FERNANDO A.; BOF BUFON, CARLOS CESAR; MAZALI, ITALO ODONE. Silicon Microchannel-Driven Raman Scattering Enhancement to Improve Gold Nanorod Functions as a SERS Substrate toward Single-Molecule Detection. ACS APPLIED MATERIALS & INTERFACES, v. 13, n. 30, p. 36482-36491, . (14/25979-2, 14/50906-9, 18/18136-0, 13/22127-2)
FINGOLO, ANA C.; DE MORAIS, VITORIA B.; COSTA, V, SAIONARA; CORREA, CATIA C.; LODI, BEATRIZ; SANTHIAGO, MURILO; BERNARDES, JULIANA S.; BUFON, CARLOS C. B.. Enhanced Hydrophobicity in Nanocellulose-Based Materials: Toward Green Wearable Devices. ACS APPLIED BIO MATERIALS, v. 4, n. 9, p. 6682-6689, . (14/25979-2, 16/04514-7, 14/50906-9)
MERCES, LEANDRO; CANDIOTTO, GRAZIANI; MINATOGAU FERRO, LETICIA MARIE; DE BARROS, ANERISE; SANTOS BATISTA, CARLOS VINICIUS; NAWAZ, ALI; RIUL JR, ANTONIO; CAPAZ, RODRIGO B.; BOF BUFON, CARLOS CESAR. Reorganization Energy upon Controlled Intermolecular Charge-Transfer Reactions in Monolithically Integrated Nanodevices. SMALL, v. 17, n. 45, . (14/25979-2, 18/18136-0, 14/50906-9, 19/10188-3, 17/02317-2, 17/21117-4, 19/14949-9)
DA SILVA, RICARDO M. L.; ALBANO, LUIZ G. S.; VELLO, TATIANA P.; DE ARAUJO, WAGNER W. R.; DE CAMARGO, DAVI H. S.; PALERMO, LEIRSON D.; CORREA, CATIA C.; WOELL, CHRISTOF; BUFON, CARLOS C. B.. Surface-Supported Metal-Organic Framework as Low-Dielectric-Constant Thin Films for Novel Hybrid Electronics. ADVANCED ELECTRONIC MATERIALS, v. N/A, p. 12-pg., . (16/25346-5, 14/25979-2, 17/02317-2, 17/25553-3, 14/50906-9)
MERCES, LEANDRO; DE OLIVEIRA, RAFAEL FURLAN; BOF BUFON, CARLOS CESAR. Nanoscale Variable-Area Electronic Devices: Contact Mechanics and Hypersensitive Pressure Application. ACS APPLIED MATERIALS & INTERFACES, v. 10, n. 45, p. 39168-39176, . (14/25979-2, 13/22127-2)
BREGADIOLLI, BRUNA ANDRESSA; PAULIN, JOAO VITOR; ALBANO, LUIZ GUSTAVO SIMAO; MARTINS, LUCAS MICHELAO; DE CAMARGO, DAVI HENRIQUE STARNINI; DA SILVA-FILHO, LUIZ CARLOS; BUFON, CARLOS CESAR BOF; GRAEFF, CARLOS FREDERICO DE OLIVEIRA. A strategy towards melanin-based functional material: rGO and sulfonated melanin composites. JOURNAL OF MATERIALS CHEMISTRY C, v. 9, n. 47, . (17/07627-0, 18/09235-4, 13/07296-2, 14/25979-2, 17/25553-3, 15/23000-1)
BARCELOS, INGRID D.; CADORE, ALISSON R.; ALENCAR, ANANIAS B.; MAIA, FRANCISCO C. B.; MANIA, EDRIAN; OLIVEIRA, RAFAEL F.; BUFON, CARLOS C. B.; MALACHIAS, ANGELO; FREITAS, RAUL O.; MOREIRA, ROBERTO L.; et al. Infrared Fingerprints of Natural 2D Talc and Plasmon-Phonon Coupling in Graphene-Talc Heterostructures. ACS PHOTONICS, v. 5, n. 5, p. 13-pg., . (14/25979-2)

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