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Development and application of composite electrodes based on graphite-poliurethane and graphite-silicone rubber-III: modification with carbon nanotubes and molecularly imprinted polymers

Grant number:08/03537-7
Support Opportunities:Regular Research Grants
Start date: July 01, 2008
End date: June 30, 2010
Field of knowledge:Physical Sciences and Mathematics - Chemistry - Analytical Chemistry
Principal Investigator:Éder Tadeu Gomes Cavalheiro
Grantee:Éder Tadeu Gomes Cavalheiro
Host Institution: Instituto de Química de São Carlos (IQSC). Universidade de São Paulo (USP). São Carlos , SP, Brazil
City of the host institution:São Carlos

Abstract

In this work the development of the composite electrodes based on carbon nanotubes (CNT)commingled by polymers, such as poliurethane resin and silicone rubber is proposed. The CNT are nanostructures with interesting properties from the viewpoint of the electrochemical sensors. They combine high superficial area, high electrical conductivity, chemical stability and mechanical strength. In principle, the CNT must present better electrochemical reversibility, low capacitive current, easy surface renovation and finally, possibility of incorporation of modifiers. It is also proposed the synthesis of the molecularly imprinted polymers (MIP) to be used in the modification of composite electrodes graphite-poliurethane for determination and quantification of analytes in complex matrices such as biological or environmental samples. This project will contribute to the development of methods for determination of substances of biological or pharmacological interest, such as paracetamol, rutin, propranolol, among others, using the modified composite electrodes. The modification of composite should give better sensitivity and selectivity to the electrodes. (AU)

Articles published in Agência FAPESP Newsletter about the research grant:
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Scientific publications (13)
(The scientific publications listed on this page originate from the Web of Science or SciELO databases. Their authors have cited FAPESP grant or fellowship project numbers awarded to Principal Investigators or Fellowship Recipients, whether or not they are among the authors. This information is collected automatically and retrieved directly from those bibliometric databases.)
SOUSA, ROGERIO A.; DOS-SANTOS, SIDNEY X.; CAVALHEIRO, EDER T. G.; BRETT, CHRISTOPHER M. A.. Graphite-Polyurethane and Graphite-Silicone Rubber Composite Electrodes for Electrochemical Characterization and Determination of Minoxidil. Electroanalysis, v. 25, n. 3, SI, p. 706-715, . (08/03537-7)
CALIXTO, CAROLINA M. F.; CERVINI, PRISCILA; CAVALHEIRO, EDER T. G.. Determination of atenolol in environmental water samples and pharmaceutical formulations at a graphite-epoxy composite electrode. INTERNATIONAL JOURNAL OF ENVIRONMENTAL ANALYTICAL CHEMISTRY, v. 92, n. 5, p. 561-570, . (08/03537-7)
DOS SANTOS, SIDNEY XAVIER; CAVALHEIRO, EDER T. G.; BRETT, CHRISTOPHER M. A.. Analytical Potentialities of Carbon Nanotube/Silicone Rubber Composite Electrodes: Determination of Propranolol. Electroanalysis, v. 22, n. 23, p. 2776-2783, . (08/03537-7)
CESARINO, IVANA; MARINO, GLIMALDO; GOMES CAVALHEIRO, EDER TADEU. A novel graphite-polyurethane composite electrode modified with thiol-organofunctionalized silica for the determination of copper ions in ethanol fuel. FUEL, v. 89, n. 8, p. 1883-1888, . (08/03537-7)
SOUSA, ROGERIO A.; DOS-SANTOS, SIDNEY X.; CAVALHEIRO, EDER T. G.; BRETT, CHRISTOPHER M. A.. Graphite-Polyurethane and Graphite-Silicone Rubber Composite Electrodes for Electrochemical Characterization and Determination of Minoxidil. Electroanalysis, v. 25, n. 3, p. 10-pg., . (08/03537-7)
CESARINO, IVANA; GOMES CAVALHEIRO, EDER TADEU. Characterization of Thiol-Functionalised Silica Films Deposited on Electrode Surfaces. MATERIALS RESEARCH-IBERO-AMERICAN JOURNAL OF MATERIALS, v. 11, n. 4, p. 465-469, . (08/03537-7)
IVANA CESARINO; ÉDER TADEU GOMES CAVALHEIRO. Characterization of thiol-functionalised silica films deposited on electrode surfaces. MATERIALS RESEARCH-IBERO-AMERICAN JOURNAL OF MATERIALS, v. 11, n. 4, p. 465-469, . (08/03537-7)
DE SOUSA, ROGERIO ADELINO; SEMAAN, FELIPE SILVA; CERVINI, PRISCILA; GOMES CAVALHEIRO, EDER TADEU. Determination of Minoxidil by Bleaching the Permanganate Carrier Solution in a Flow-Based Spectrophotometric System. Analytical Letters, v. 44, n. 1-3, p. 349-359, . (08/03537-7)
CERVINI, PRISCILA; GOMES CAVALHEIRO, EDER TADEU. Evaluation of the Analytical Potentialities of a Composite Electrode Modified with Molecularly Imprinted Polymers. Analytical Letters, v. 42, n. 13, p. 1940-1957, . (08/03537-7, 06/06133-9)
CESARINO, IVANA; GOUVEIA-CARIDADE, CARLA; PAULIUKAITE, RASA; CAVALHEIRO, EDER T. G.; BRETT, CHRISTOPHER M. A.. Characterization and Application of Bismuth-Film Modified Graphite-Polyurethane Composite Electrodes. Electroanalysis, v. 22, n. 13, p. 1437-1445, . (08/03537-7)
CESARINO, IVANA; GOMES CAVALHEIRO, EDER TADEU. Characterization of Thiol-Functionalised Silica Films Deposited on Electrode Surfaces. MATERIALS RESEARCH-IBERO-AMERICAN JOURNAL OF MATERIALS, v. 11, n. 4, p. 5-pg., . (08/03537-7)